Faraday Discuss., 2023, 245,52-79
DOI: 10.1039/D3FD00010A, Paper

Ewine F. van Dishoeck, S. Grant, B. Tabone, M. van Gelder, L. Francis, L. Tychoniec, G. Bettoni, A. M. Arabhavi, D. Gasman, P. Nazari, M. Vlasblom, P. Kavanagh, V. Christiaens, P. Klaassen, H. Beuther, Th. Henning, I. Kamp
Early results from JWST-MIRI programs on low- and high-mass protostars and disks show significant diversity in their mid-infrared spectra, most notably for CO₂, H₂O and C₂H₂. Benzene is detected in disks around very low mass stars.
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Faraday Discuss., 2023, Advance Article
DOI: 10.1039/D3FD00088E, Paper

Open Access

  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.

Soumyadip Mondal, Rajesh B. Jethwa, Bhargavi Pant, Robert Hauschild, Stefan A. Freunberger
We have shown direct spectroscopic evidence of the previously identified pathways for singlet oxygen (¹O₂) formation in non-aqueous oxygen redox chemistry.
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Faraday Discuss., 2023, Advance Article
DOI: 10.1039/D3FD00096F, Paper

Pierre L. Stigliano, Nagore Ortiz-Vitoriano, Lidia Medinilla, Jason E. Bara, Juan Miguel López del Amo, Luis Lezama, Maria Forsyth, David Mecerreyes, Cristina Pozo-Gonzalo
A green, low-toxic diglyme isomer, 1,2,3-trimethoxypropane, has been studied, for the first time, as the electrolyte in sodium–air batteries reaching 2.31 mA h cm⁻² discharge capacity and with NaO₂ as the main discharge product.
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Faraday Discuss., 2023, Advance Article
DOI: 10.1039/D3FD00079F, Paper

Kiwoong Lee, Jeff Sakamoto
This study demonstrates that the stability of cycling in situ Li anodes depends on their depth of discharge (DOD). High DOD cycling results in unstable performance due to the accumulation of interfacial degradation at Li/LLZO interfaces.
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Faraday Discuss., 2023, 245,11-51
DOI: 10.1039/D3FD00106G, Paper

Open Access

  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.

Cecilia Ceccarelli
This Spiers Memorial Lecture introduces the Faraday Discussion on ‘Astrochemistry at high resolution’, focusing on the special case of interstellar complex organic molecules (iCOMs).
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Faraday Discuss., 2023, Advance Article
DOI: 10.1039/D3FD00093A, Paper

Open Access

  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.

Giada Franceschi, Sebastian Brandstetter, Jan Balajka, Igor Sokolović, Jiří Pavelec, Martin Setvín, Michael Schmid, Ulrike Diebold
XPS and atomically resolved nc-AFM shed light on the interaction of the surface K⁺ ions of muscovite mica with water vapor and liquid water under ultraclean conditions.
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Faraday Discuss., 2023, 245,368-379
DOI: 10.1039/D3FD00019B, Paper

D. Michelle Bailey, Eric M. Crump, Joseph T. Hodges, Adam J. Fleisher
Direct frequency comb spectroscopy of HCN is performed using a high resolution, cross-dispersed spectrometer. Short-wave and mid-wave infrared instrumentation for precision molecular spectroscopy to test line lists is discussed.
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Faraday Discuss., 2023, 245,569-585
DOI: 10.1039/D3FD00008G, Paper

Johannes Heyl, Serena Viti, Gijs Vermariën
We use Bayesian inference together with the MOPED compression algorithm to help determine which species should be prioritised for future detections in order to better constrain the values of binding energies in the ISM.
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Faraday Discuss., 2023, Advance Article
DOI: 10.1039/D3FD00083D, Paper

Nannan Shan, Anh T. Ngo, Alireza Kondari, Mohammad Asadi, Larry A. Curtiss
Calculated interface between Li₂O and Li₂O₂ surfaces showing the extent of disorder at the interface. Such interfaces are probably present in the new solid-state Li–air battery described here and contribute to the discharge and charge mechanisms.
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Faraday Discuss., 2023, Advance Article
DOI: 10.1039/D3FD00103B, Paper

Jean-François Olivieri, James T. Hynes, Damien Laage
We perform molecular dynamics simulations of aqueous NaCl solutions at the interface with graphene electrodes, and examine the impact of both ion concentration and electrode potential on interfacial water reorientational dynamics.
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